Transmutation of nuclear wastes using photonuclear reactions triggered by Compton backscattering photons at the Shanghai laser electron gamma source

CHEN Jin-Gen; XU Wang; WANG Hong-Wei; GUO Wei; MA Yu-Gang; CAI Xiang-Zhou; LU Guang-Cheng; XU Yi; PAN Qiang-Yan; YUAN Ren-Yong; XU Jia-Qiang; YAN Zhe; FAN Gong-Tao; SHEN Wen-Qing

doi:10.1088/1674-1137/32/8/019

Chinese Physics C> 2008, Vol. 32> Issue(8) : 677-680 DOI: 10.1088/1674-1137/32/8/019

Transmutation of nuclear wastes using photonuclear reactions triggered by Compton backscattering photons at the Shanghai laser electron gamma source

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Abstract：
Based on the facility of the Shanghai Laser Electron Gamma Source (SLEGS), the transmutation for nuclear wastes such as ¹³⁷Cs and ¹²⁹I is investigated. It is found that nuclear waste can be transmuted efficiently via photonuclear reaction triggered by gamma photons generated from Compton backscattering between CO₂ laser photons and 3.5 GeV electrons. The nuclear activities of ¹³⁷Cs and ¹²⁹I are evaluated and compared with the results of transmutation triggered by bremsstrahlung gamma photons driven by ultra intense laser. Due to the better character of gamma photon spectrum as well as the high brightness of gamma photons, the transmutation rate of Compton backscattering method is much higher than that of the bremsstrahlung method.

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[1]

. Michel R, Klipsch K, Ernst Th et al. Radioprotection, 2005,40(Suppl.1): S2692. Baetslé L H, Achuthan P V, Burcl R et al. Implications of Partitioning and Transmutation in Radioactive Waste Management. Vienna: International Atomic Energy Agency Press, 20033. Yiou F, Raisbeck G M, ZHOU Z Q et al. Nucl. Instrum.Methods B, 1994, 92: 4364. Rubbia C, Abderrahim H A, Bjornberg M et al. A European Roadmap for Developing Accelerator Driven Systemsfor Nuclear Waste Incineration. Roma: ENEA Publishers,20015. Harada H, Sekine T, Hatsukawa Y et al. J. Nucl. Sci. Tech.,1994, 31: 1736. Harada H, Watanabe H, Sekine T et al. J. Nucl. Sci. Tech.,1990, 27: 5777. CAI D F, GU Y Q, ZHENG Z J et al. Chin. Phys., 2006,15: 23638. XU M H, LIANG T J, ZHANG J. Acta Phys. Sin., 2006,55: 2357 (in Chinese)9. Shkolnikova P L, Kaplan A E, Pukhov A et al. Appl. Phys.Lett., 1997, 71: 347310. Norreys P A, Santala M, Clark E et al. Phys. Plasmas,1999, 6: 215011. Malka V, Fritzler S, Lefebvre E et al. Science, 2002, 22:159612. Ledingham K W D, Magill J, McKenna P et al. J. Phys.D, 2003, 36: L7913. Magill J, Schwoerer H, Ewald F et al. Appl. Phys. B, 2003,77: 38714. Liesfeld B, Amthor K U, Ewald F et al. Appl. Phys. B,2004, 79: 104715. Sadighi-bonabi R, Kokabee O. Chin. Phys. Lett., 2006, 23:143416. Balakin V, Alexandrov V A, Mikhailichenko A et al. Phys.Rev. Lett., 1995, 74: 247917. Imasaki K, Moon A. Int. Soc. Opt. Eng., 2000, 3886: 72118. GUO W, XU W, CHEN J G et al. Nucl. Instrum. MethodsA, 2007, 578: 45719. Bandazhevskaya G S, Nesterenko V B, Babenko V I et al.Swiss Med Wkly, 2004, 134: 72520. ZHAO Z T, XU H J. SSRF: A 3.5 GeV Synchrotron Light Source for China. In: Europen Physcial Society Accelerator Group ed. Proceeding of EPAC 2004. Lucerne: PaulScherrer Institute Press, 2004. 236821. Klein O, Nishina Y. Z. Physik, 1929, 52: 85322. Handbook on Photonuclear Data for Applications-Cross Sections and Spectra. Vienna: International Atomic Energy Agency Press, 2000

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CHEN Jin-Gen, XU Wang, WANG Hong-Wei, GUO Wei, MA Yu-Gang, CAI Xiang-Zhou, LU Guang-Cheng, XU Yi, PAN Qiang-Yan, YUAN Ren-Yong, XU Jia-Qiang, YAN Zhe, FAN Gong-Tao and SHEN Wen-Qing. Transmutation of nuclear wastes using photonuclear reactions triggered by Compton backscattering photons at the Shanghai laser electron gamma source[J]. Chinese Physics C, 2008, 32(8): 677-680. doi: 10.1088/1674-1137/32/8/019

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Received: 2007-10-11
Revised: 2007-11-04

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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Transmutation of nuclear wastes using photonuclear reactions triggered by Compton backscattering photons at the Shanghai laser electron gamma source

Corresponding author: CHEN Jin-Gen,

Received Date: 2007-10-11

Accepted Date: 2007-11-04

Available Online: 2008-08-05

Abstract:

Based on the facility of the Shanghai Laser Electron Gamma Source (SLEGS), the transmutation for nuclear wastes such as ¹³⁷Cs and ¹²⁹I is investigated. It is found that nuclear waste can be transmuted efficiently via photonuclear reaction triggered by gamma photons generated from Compton backscattering between CO₂ laser photons and 3.5 GeV electrons. The nuclear activities of ¹³⁷Cs and ¹²⁹I are evaluated and compared with the results of transmutation triggered by bremsstrahlung gamma photons driven by ultra intense laser. Due to the better character of gamma photon spectrum as well as the high brightness of gamma photons, the transmutation rate of Compton backscattering method is much higher than that of the bremsstrahlung method.

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Transmutation of nuclear wastes using photonuclear reactions triggered by Compton backscattering photons at the Shanghai laser electron gamma source

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